The Collaborative International Dictionary of English v.0.48:
Brain \Brain\ (br[=a]n), v. t. [imp. & p. p. Brained
(br[=a]nd); p. pr. & vb. n. Braining.]
[1913 Webster]
1. To dash out the brains of; to kill by beating out the
brains. Hence, Fig.: To destroy; to put an end to; to
defeat.
[1913 Webster]
There thou mayst brain him. --Shak.
[1913 Webster]
It was the swift celerity of the death . . .
That brained my purpose. --Shak.
[1913 Webster]
2. To conceive; to understand. [Obs.]
[1913 Webster]
'T is still a dream, or else such stuff as madmen
Tongue, and brain not. --Shak.
[1913 Webster]