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The Collaborative International Dictionary of English v.0.48:

Polysyllabic \Pol`y*syl*lab"ic\, Polysyllabical
\Pol`y*syl*lab"ic*al\, a. [Gr. ?; poly`s many + ? syllable: cf.
   F. polysyllabique.]
   Pertaining to a polysyllable; containing, or characterized
   by, polysyllables; consisting of more than three syllables.
   [1913 Webster]