The Collaborative International Dictionary of English v.0.48:
Toughen \Tough"en\, v. i. & t. [imp. & p. p. Toughened; p. pr. & vb. n. Toughening.] To grow or make tough, or tougher. [1913 Webster]WordNet (r) 3.0 (2006):
toughen v 1: make tough or tougher; "This experience will toughen her"