The Collaborative International Dictionary of English v.0.48:
Unbridle \Un*bri"dle\, v. t. [1st pref. un- + bridle.] To free from the bridle; to set loose. [1913 Webster]WordNet (r) 3.0 (2006):
unbridle v 1: remove the bridle from (a horse or mule) [ant: bridle]